Ultrafast dissociation processes in the NO dimer studied with time-resolved photoelectron imaging
Lange, C.A. de
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1 ps to the dimer 3s Rydberg state. This dimer Rydberg state then undergoes fragmentation on a time scale of a few ps. In this study we focus on dissociation into an NO ground state fragment and an NO fragment in its 3s Rydberg A(2)Sigma(+) state. Every stage of this continuous process, viz. the dimer valence state, the dimer 3s Rydberg state, the separating NO(X) + NO(A) fragments, and the isolated NO(A) fragment is interrogated with TR-PEI. (C) 2004 Elsevier B.V. All rights reserved.